Progress in understanding and development of Ba0.5Sr0.5Co0.8Fe0.2O3−δ-based cathodes for intermediate-temperature solid-oxide fuel cells: A review

Solid-oxide fuel cells (SOFCs) convert chemical energy directly into electric power in a highly efficient way. Lowering the operating temperature of SOFCs to around 500-800 °C is one of the main goals in current SOFC research. The associated benefits include reducing the difficulties associated with...

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Main Authors: Zhou, W., Ran, R., Shao, Zongping
Format: Journal Article
Published: Elsevier SA 2009
Online Access:http://hdl.handle.net/20.500.11937/21651
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author Zhou, W.
Ran, R.
Shao, Zongping
author_facet Zhou, W.
Ran, R.
Shao, Zongping
author_sort Zhou, W.
building Curtin Institutional Repository
collection Online Access
description Solid-oxide fuel cells (SOFCs) convert chemical energy directly into electric power in a highly efficient way. Lowering the operating temperature of SOFCs to around 500-800 °C is one of the main goals in current SOFC research. The associated benefits include reducing the difficulties associated with sealing and thermal degradation, allowing the use of low-cost metallic interconnectors and suppressing reactions between the cell components. However, the electrochemical activity of the cathode deteriorates dramatically with decreasing temperature for the typical La0.8Sr0.2MnO3-based electrodes. The cathode becomes the limiting factor in determining the overall cell performance. Therefore, the development of new electrodes with high electrocatalytic activity for oxygen reduction becomes a critical issue for intermediate-temperature (IT)-SOFCs. Ba0.5Sr0.5Co0.8Fe0.2O3-d (BSCF) perovskite oxide was first reported as a potential IT-SOFC cathode material in 2004 by Shao and Haile. After that, the BSCF cathode has attracted considerable attention. This paper reviews the current research activities on BSCF-based cathodes for IT-SOFCs. Emphasis will be placed on the understanding and optimization of BSCF-based materials. The issues raised by the BSCF cathode are also presented and analyzed to provide some guidelines in the search for the new generation of cathode materials for IT-SOFCs. © 2009 Elsevier B.V. All rights reserved.
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spelling curtin-20.500.11937-216512017-09-13T13:55:43Z Progress in understanding and development of Ba0.5Sr0.5Co0.8Fe0.2O3−δ-based cathodes for intermediate-temperature solid-oxide fuel cells: A review Zhou, W. Ran, R. Shao, Zongping Solid-oxide fuel cells (SOFCs) convert chemical energy directly into electric power in a highly efficient way. Lowering the operating temperature of SOFCs to around 500-800 °C is one of the main goals in current SOFC research. The associated benefits include reducing the difficulties associated with sealing and thermal degradation, allowing the use of low-cost metallic interconnectors and suppressing reactions between the cell components. However, the electrochemical activity of the cathode deteriorates dramatically with decreasing temperature for the typical La0.8Sr0.2MnO3-based electrodes. The cathode becomes the limiting factor in determining the overall cell performance. Therefore, the development of new electrodes with high electrocatalytic activity for oxygen reduction becomes a critical issue for intermediate-temperature (IT)-SOFCs. Ba0.5Sr0.5Co0.8Fe0.2O3-d (BSCF) perovskite oxide was first reported as a potential IT-SOFC cathode material in 2004 by Shao and Haile. After that, the BSCF cathode has attracted considerable attention. This paper reviews the current research activities on BSCF-based cathodes for IT-SOFCs. Emphasis will be placed on the understanding and optimization of BSCF-based materials. The issues raised by the BSCF cathode are also presented and analyzed to provide some guidelines in the search for the new generation of cathode materials for IT-SOFCs. © 2009 Elsevier B.V. All rights reserved. 2009 Journal Article http://hdl.handle.net/20.500.11937/21651 10.1016/j.jpowsour.2009.02.069 Elsevier SA restricted
spellingShingle Zhou, W.
Ran, R.
Shao, Zongping
Progress in understanding and development of Ba0.5Sr0.5Co0.8Fe0.2O3−δ-based cathodes for intermediate-temperature solid-oxide fuel cells: A review
title Progress in understanding and development of Ba0.5Sr0.5Co0.8Fe0.2O3−δ-based cathodes for intermediate-temperature solid-oxide fuel cells: A review
title_full Progress in understanding and development of Ba0.5Sr0.5Co0.8Fe0.2O3−δ-based cathodes for intermediate-temperature solid-oxide fuel cells: A review
title_fullStr Progress in understanding and development of Ba0.5Sr0.5Co0.8Fe0.2O3−δ-based cathodes for intermediate-temperature solid-oxide fuel cells: A review
title_full_unstemmed Progress in understanding and development of Ba0.5Sr0.5Co0.8Fe0.2O3−δ-based cathodes for intermediate-temperature solid-oxide fuel cells: A review
title_short Progress in understanding and development of Ba0.5Sr0.5Co0.8Fe0.2O3−δ-based cathodes for intermediate-temperature solid-oxide fuel cells: A review
title_sort progress in understanding and development of ba0.5sr0.5co0.8fe0.2o3−δ-based cathodes for intermediate-temperature solid-oxide fuel cells: a review
url http://hdl.handle.net/20.500.11937/21651