Response of a copper (II) and iron (III) ion-selective electrode bielectrode array in saline media

A bielectrode array comprising a jalpaite membrane (i.e., Ag1.5Cu0.5S) copper(II) ion-selective electrode (ISE) and chalcogenide glass membrane (i.e., Fe2.5(Se60Ge28Sb12)97.5) iron(III) ISE has been assembled by individually wiring each solid-state sensor into a single electrode body.Furthermore, a...

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Main Authors: De Marco, Roland, Martizano, Jay
Format: Journal Article
Published: Elsevier 2008
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/21552
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author De Marco, Roland
Martizano, Jay
author_facet De Marco, Roland
Martizano, Jay
author_sort De Marco, Roland
building Curtin Institutional Repository
collection Online Access
description A bielectrode array comprising a jalpaite membrane (i.e., Ag1.5Cu0.5S) copper(II) ion-selective electrode (ISE) and chalcogenide glass membrane (i.e., Fe2.5(Se60Ge28Sb12)97.5) iron(III) ISE has been assembled by individually wiring each solid-state sensor into a single electrode body.Furthermore, a dual metal ion buffer calibration standard incorporating copper(II) and iron(III) coordinating ligands to regulate the levels of free copper(II) and iron(III) in the buffer has been developed to enable simultaneous calibration of the bielectrode ISE array. In this work, the bielectrodeISE array has been employed in the continuous flow analysis (CFA) of free copper(II) and iron(III) in seawater media. It is shown that the individual electrodes displayed Nernstian response in the metal ion buffer calibration standard over a wide dynamic range (viz., 10-15 to 10-5M aCu2+ and10-21 to 10-11M aFe3+), and the results of repetitive CFA analyses of free copper(II) and iron(III) in seawater are commensurate with the typical values found in coastal seawater samples. Clearly, the bielectrode ISE array may be used in the simultaneous analysis of free copper(II) and iron(III)in seawater without fear of cross-interference between the solid-state sensors.
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spelling curtin-20.500.11937-215522018-10-02T05:21:52Z Response of a copper (II) and iron (III) ion-selective electrode bielectrode array in saline media De Marco, Roland Martizano, Jay Ion-selective electrode Seawater Copper and iron Metal speciation Trace metals A bielectrode array comprising a jalpaite membrane (i.e., Ag1.5Cu0.5S) copper(II) ion-selective electrode (ISE) and chalcogenide glass membrane (i.e., Fe2.5(Se60Ge28Sb12)97.5) iron(III) ISE has been assembled by individually wiring each solid-state sensor into a single electrode body.Furthermore, a dual metal ion buffer calibration standard incorporating copper(II) and iron(III) coordinating ligands to regulate the levels of free copper(II) and iron(III) in the buffer has been developed to enable simultaneous calibration of the bielectrode ISE array. In this work, the bielectrodeISE array has been employed in the continuous flow analysis (CFA) of free copper(II) and iron(III) in seawater media. It is shown that the individual electrodes displayed Nernstian response in the metal ion buffer calibration standard over a wide dynamic range (viz., 10-15 to 10-5M aCu2+ and10-21 to 10-11M aFe3+), and the results of repetitive CFA analyses of free copper(II) and iron(III) in seawater are commensurate with the typical values found in coastal seawater samples. Clearly, the bielectrode ISE array may be used in the simultaneous analysis of free copper(II) and iron(III)in seawater without fear of cross-interference between the solid-state sensors. 2008 Journal Article http://hdl.handle.net/20.500.11937/21552 10.1016/j.talanta.2008.01.018 Elsevier fulltext
spellingShingle Ion-selective electrode
Seawater
Copper and iron
Metal speciation
Trace metals
De Marco, Roland
Martizano, Jay
Response of a copper (II) and iron (III) ion-selective electrode bielectrode array in saline media
title Response of a copper (II) and iron (III) ion-selective electrode bielectrode array in saline media
title_full Response of a copper (II) and iron (III) ion-selective electrode bielectrode array in saline media
title_fullStr Response of a copper (II) and iron (III) ion-selective electrode bielectrode array in saline media
title_full_unstemmed Response of a copper (II) and iron (III) ion-selective electrode bielectrode array in saline media
title_short Response of a copper (II) and iron (III) ion-selective electrode bielectrode array in saline media
title_sort response of a copper (ii) and iron (iii) ion-selective electrode bielectrode array in saline media
topic Ion-selective electrode
Seawater
Copper and iron
Metal speciation
Trace metals
url http://hdl.handle.net/20.500.11937/21552