Effectiveness of Ferric Salts to Remove Low Levels of Dosed Copper from NOM-Containing Natural Water

Water utilities dose copper in drinking water systems to inhibit/kill microorganisms including algae. Under conditions observed in the systems, the majority of dosed copper is reported to be in dissolved forms of Cu-NOM and inorganic compounds. High concentrations (40 mg/L) of ferric salts are repor...

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Main Authors: Zhan, Weixi, Sathasivan, Arumugam, Nolan, P., Koska, L., Heitz, Anna, Joll, Cynthia
Other Authors: TBA
Format: Journal Article
Published: IWA Publishing 2009
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/19754
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author Zhan, Weixi
Sathasivan, Arumugam
Nolan, P.
Koska, L.
Heitz, Anna
Joll, Cynthia
author2 TBA
author_facet TBA
Zhan, Weixi
Sathasivan, Arumugam
Nolan, P.
Koska, L.
Heitz, Anna
Joll, Cynthia
author_sort Zhan, Weixi
building Curtin Institutional Repository
collection Online Access
description Water utilities dose copper in drinking water systems to inhibit/kill microorganisms including algae. Under conditions observed in the systems, the majority of dosed copper is reported to be in dissolved forms of Cu-NOM and inorganic compounds. High concentrations (40 mg/L) of ferric salts are reported to be able to remove large amounts of copper. However, the fate of dissolved copper when a small amount of ferric salts (<2 mg/L) is present in natural water or in the distribution pipes when they are released from the corroded iron pipes are not known. The current paper investigates the mechanisms behind the dissolved copper removal in NOM-containing bulk water. When copper was dosed from 250–800 mg-Cu/L, relatively high solubility was demonstrated in Mundaring water, with dissolved copper increased from 250–720 mg-Cu/L. Both ferric chloride and ferric hydroxide were found to have a considerable ability to remove dissolved copper while the former showed higher capacity. Ferric chloride showed a linear relationship with copper removal (R2=0.99) and the removal by ferric hydroxide showed excellent agreement with either the Freundlich (R2=0.98) or Langmuir (R2=0.99) adsorption isotherm.
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spelling curtin-20.500.11937-197542017-09-13T16:00:43Z Effectiveness of Ferric Salts to Remove Low Levels of Dosed Copper from NOM-Containing Natural Water Zhan, Weixi Sathasivan, Arumugam Nolan, P. Koska, L. Heitz, Anna Joll, Cynthia TBA Langmuir isotherm copper NOM Freundlich isotherm ferric salts adsorption Water utilities dose copper in drinking water systems to inhibit/kill microorganisms including algae. Under conditions observed in the systems, the majority of dosed copper is reported to be in dissolved forms of Cu-NOM and inorganic compounds. High concentrations (40 mg/L) of ferric salts are reported to be able to remove large amounts of copper. However, the fate of dissolved copper when a small amount of ferric salts (<2 mg/L) is present in natural water or in the distribution pipes when they are released from the corroded iron pipes are not known. The current paper investigates the mechanisms behind the dissolved copper removal in NOM-containing bulk water. When copper was dosed from 250–800 mg-Cu/L, relatively high solubility was demonstrated in Mundaring water, with dissolved copper increased from 250–720 mg-Cu/L. Both ferric chloride and ferric hydroxide were found to have a considerable ability to remove dissolved copper while the former showed higher capacity. Ferric chloride showed a linear relationship with copper removal (R2=0.99) and the removal by ferric hydroxide showed excellent agreement with either the Freundlich (R2=0.98) or Langmuir (R2=0.99) adsorption isotherm. 2009 Journal Article http://hdl.handle.net/20.500.11937/19754 10.2166/aqua.2009.006 IWA Publishing restricted
spellingShingle Langmuir isotherm
copper
NOM
Freundlich isotherm
ferric salts
adsorption
Zhan, Weixi
Sathasivan, Arumugam
Nolan, P.
Koska, L.
Heitz, Anna
Joll, Cynthia
Effectiveness of Ferric Salts to Remove Low Levels of Dosed Copper from NOM-Containing Natural Water
title Effectiveness of Ferric Salts to Remove Low Levels of Dosed Copper from NOM-Containing Natural Water
title_full Effectiveness of Ferric Salts to Remove Low Levels of Dosed Copper from NOM-Containing Natural Water
title_fullStr Effectiveness of Ferric Salts to Remove Low Levels of Dosed Copper from NOM-Containing Natural Water
title_full_unstemmed Effectiveness of Ferric Salts to Remove Low Levels of Dosed Copper from NOM-Containing Natural Water
title_short Effectiveness of Ferric Salts to Remove Low Levels of Dosed Copper from NOM-Containing Natural Water
title_sort effectiveness of ferric salts to remove low levels of dosed copper from nom-containing natural water
topic Langmuir isotherm
copper
NOM
Freundlich isotherm
ferric salts
adsorption
url http://hdl.handle.net/20.500.11937/19754