Development of Novel Alkoxyisoxazoles as Sigma-1 Receptor Antagonists with Antinociceptive Efficacy

A novel series of sigma (s) receptor ligands based on an alkoxyisoxazole scaffold has been designed and synthesized. Preliminary receptor binding assays identified highly potent (Ki < 1 nM) and selective s1 ligands devoid of binding interactions with the monoamine transporters DAT, NET, and SERT....

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Main Authors: Sun, H., Shi, M., Zhang, W., Zheng, Y., Xu, Y., Shi, J., Liu, T., Gunosewoyo, Hendra, Pang, T., Gao, Z., Yang, F., Tang, J., Yu, L.
Format: Journal Article
Published: American Chemical Society 2016
Online Access:http://hdl.handle.net/20.500.11937/18018
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author Sun, H.
Shi, M.
Zhang, W.
Zheng, Y.
Xu, Y.
Shi, J.
Liu, T.
Gunosewoyo, Hendra
Pang, T.
Gao, Z.
Yang, F.
Tang, J.
Yu, L.
author_facet Sun, H.
Shi, M.
Zhang, W.
Zheng, Y.
Xu, Y.
Shi, J.
Liu, T.
Gunosewoyo, Hendra
Pang, T.
Gao, Z.
Yang, F.
Tang, J.
Yu, L.
author_sort Sun, H.
building Curtin Institutional Repository
collection Online Access
description A novel series of sigma (s) receptor ligands based on an alkoxyisoxazole scaffold has been designed and synthesized. Preliminary receptor binding assays identified highly potent (Ki < 1 nM) and selective s1 ligands devoid of binding interactions with the monoamine transporters DAT, NET, and SERT. In particular, compound 53 was shown to possess significant antinociceptive activity in the mouse formalin-induced inflammation pain model when administered intraperitoneally at 40 and 80 mg/kg. Initial pharmacokinetics evaluation indicated an excellent brain exposure following oral dosing in mice, suggesting that further investigation into the use of alkoxyisoxazoles as s1 ligands for antinociception is warranted. This study supports the notion that selective s1 antagonism could be a useful strategy in the development of novel antipain therapy.
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institution Curtin University Malaysia
institution_category Local University
last_indexed 2025-11-14T07:23:54Z
publishDate 2016
publisher American Chemical Society
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spelling curtin-20.500.11937-180182017-09-13T15:44:54Z Development of Novel Alkoxyisoxazoles as Sigma-1 Receptor Antagonists with Antinociceptive Efficacy Sun, H. Shi, M. Zhang, W. Zheng, Y. Xu, Y. Shi, J. Liu, T. Gunosewoyo, Hendra Pang, T. Gao, Z. Yang, F. Tang, J. Yu, L. A novel series of sigma (s) receptor ligands based on an alkoxyisoxazole scaffold has been designed and synthesized. Preliminary receptor binding assays identified highly potent (Ki < 1 nM) and selective s1 ligands devoid of binding interactions with the monoamine transporters DAT, NET, and SERT. In particular, compound 53 was shown to possess significant antinociceptive activity in the mouse formalin-induced inflammation pain model when administered intraperitoneally at 40 and 80 mg/kg. Initial pharmacokinetics evaluation indicated an excellent brain exposure following oral dosing in mice, suggesting that further investigation into the use of alkoxyisoxazoles as s1 ligands for antinociception is warranted. This study supports the notion that selective s1 antagonism could be a useful strategy in the development of novel antipain therapy. 2016 Journal Article http://hdl.handle.net/20.500.11937/18018 10.1021/acs.jmedchem.6b00571 American Chemical Society restricted
spellingShingle Sun, H.
Shi, M.
Zhang, W.
Zheng, Y.
Xu, Y.
Shi, J.
Liu, T.
Gunosewoyo, Hendra
Pang, T.
Gao, Z.
Yang, F.
Tang, J.
Yu, L.
Development of Novel Alkoxyisoxazoles as Sigma-1 Receptor Antagonists with Antinociceptive Efficacy
title Development of Novel Alkoxyisoxazoles as Sigma-1 Receptor Antagonists with Antinociceptive Efficacy
title_full Development of Novel Alkoxyisoxazoles as Sigma-1 Receptor Antagonists with Antinociceptive Efficacy
title_fullStr Development of Novel Alkoxyisoxazoles as Sigma-1 Receptor Antagonists with Antinociceptive Efficacy
title_full_unstemmed Development of Novel Alkoxyisoxazoles as Sigma-1 Receptor Antagonists with Antinociceptive Efficacy
title_short Development of Novel Alkoxyisoxazoles as Sigma-1 Receptor Antagonists with Antinociceptive Efficacy
title_sort development of novel alkoxyisoxazoles as sigma-1 receptor antagonists with antinociceptive efficacy
url http://hdl.handle.net/20.500.11937/18018