An 800-Year Record of Atmospheric As, Mo, Sn, and Sb in Central Asia in High-Altitude Ice Cores from Mt. Qomolangma (Everest), Himalayas

As, Mo, Sn, and Sb have been determined by inductively coupled plasma sector field mass spectrometry (ICP-SFMS) in 143 depth intervals of high-altitude ice cores from Mt. Everest, covering an 800-year time period from 1205 to 2002 AD. The results clearly demonstrate the long-term historical record o...

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Main Authors: Hong, S., Lee, K., Hou, S., Hur, S., Ren, J., Nunes, Laurie, Rosman, Kevin, Barbante, C., Boutron, C.
Other Authors: Bernd Zolitschka
Format: Journal Article
Published: American Chemical Society 2009
Online Access:http://hdl.handle.net/20.500.11937/17496
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author Hong, S.
Lee, K.
Hou, S.
Hur, S.
Ren, J.
Nunes, Laurie
Rosman, Kevin
Barbante, C.
Boutron, C.
author2 Bernd Zolitschka
author_facet Bernd Zolitschka
Hong, S.
Lee, K.
Hou, S.
Hur, S.
Ren, J.
Nunes, Laurie
Rosman, Kevin
Barbante, C.
Boutron, C.
author_sort Hong, S.
building Curtin Institutional Repository
collection Online Access
description As, Mo, Sn, and Sb have been determined by inductively coupled plasma sector field mass spectrometry (ICP-SFMS) in 143 depth intervals of high-altitude ice cores from Mt. Everest, covering an 800-year time period from 1205 to 2002 AD. The results clearly demonstrate the long-term historical record of atmospheric transport and deposition of As, Mo, Sn, and Sb that has prevailed at high altitudes in the central Himalayas. Natural contributions, mainly from mineral dust, have dominated the atmospheric cycles of As, Mo, Sn, and to some extent Sb during the 700 years prior to the 20th century. Compared to those of the pre-1900 period, pronounced increases of both concentrations and crustal enrichment factors are observed since the 1970s, with the highest increase factor for Sn and the lowest for As. Such increases are attributed to anthropogenic emissions of these elements, largely from stationary fossil fuel combustion and nonferrous metals production, particularly in India. Our central Himalayan ice core record provides an explicit recognition of rising atmospheric As, Mo, Sn, and Sb pollution in response to rapid economic growth in central Asia.
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publishDate 2009
publisher American Chemical Society
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spelling curtin-20.500.11937-174962017-09-13T15:44:55Z An 800-Year Record of Atmospheric As, Mo, Sn, and Sb in Central Asia in High-Altitude Ice Cores from Mt. Qomolangma (Everest), Himalayas Hong, S. Lee, K. Hou, S. Hur, S. Ren, J. Nunes, Laurie Rosman, Kevin Barbante, C. Boutron, C. Bernd Zolitschka As, Mo, Sn, and Sb have been determined by inductively coupled plasma sector field mass spectrometry (ICP-SFMS) in 143 depth intervals of high-altitude ice cores from Mt. Everest, covering an 800-year time period from 1205 to 2002 AD. The results clearly demonstrate the long-term historical record of atmospheric transport and deposition of As, Mo, Sn, and Sb that has prevailed at high altitudes in the central Himalayas. Natural contributions, mainly from mineral dust, have dominated the atmospheric cycles of As, Mo, Sn, and to some extent Sb during the 700 years prior to the 20th century. Compared to those of the pre-1900 period, pronounced increases of both concentrations and crustal enrichment factors are observed since the 1970s, with the highest increase factor for Sn and the lowest for As. Such increases are attributed to anthropogenic emissions of these elements, largely from stationary fossil fuel combustion and nonferrous metals production, particularly in India. Our central Himalayan ice core record provides an explicit recognition of rising atmospheric As, Mo, Sn, and Sb pollution in response to rapid economic growth in central Asia. 2009 Journal Article http://hdl.handle.net/20.500.11937/17496 10.1021/es901685u American Chemical Society restricted
spellingShingle Hong, S.
Lee, K.
Hou, S.
Hur, S.
Ren, J.
Nunes, Laurie
Rosman, Kevin
Barbante, C.
Boutron, C.
An 800-Year Record of Atmospheric As, Mo, Sn, and Sb in Central Asia in High-Altitude Ice Cores from Mt. Qomolangma (Everest), Himalayas
title An 800-Year Record of Atmospheric As, Mo, Sn, and Sb in Central Asia in High-Altitude Ice Cores from Mt. Qomolangma (Everest), Himalayas
title_full An 800-Year Record of Atmospheric As, Mo, Sn, and Sb in Central Asia in High-Altitude Ice Cores from Mt. Qomolangma (Everest), Himalayas
title_fullStr An 800-Year Record of Atmospheric As, Mo, Sn, and Sb in Central Asia in High-Altitude Ice Cores from Mt. Qomolangma (Everest), Himalayas
title_full_unstemmed An 800-Year Record of Atmospheric As, Mo, Sn, and Sb in Central Asia in High-Altitude Ice Cores from Mt. Qomolangma (Everest), Himalayas
title_short An 800-Year Record of Atmospheric As, Mo, Sn, and Sb in Central Asia in High-Altitude Ice Cores from Mt. Qomolangma (Everest), Himalayas
title_sort 800-year record of atmospheric as, mo, sn, and sb in central asia in high-altitude ice cores from mt. qomolangma (everest), himalayas
url http://hdl.handle.net/20.500.11937/17496