Investigation of growth rate dispersion in lactose crystallisation by AFM

α-Lactose monohydrate crystals have been reported to exhibit growth rate dispersion (GRD). Variation in surface dislocations has been suggested as the cause of GRD, but this has not been further investigated to date. In this study, growth rate dispersion and the change in morphology were investigate...

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Main Authors: Dincer, Tuna, Ogden, Mark, Parkinson, Gordon
Format: Journal Article
Published: Elsevier 2014
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/17081
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author Dincer, Tuna
Ogden, Mark
Parkinson, Gordon
author_facet Dincer, Tuna
Ogden, Mark
Parkinson, Gordon
author_sort Dincer, Tuna
building Curtin Institutional Repository
collection Online Access
description α-Lactose monohydrate crystals have been reported to exhibit growth rate dispersion (GRD). Variation in surface dislocations has been suggested as the cause of GRD, but this has not been further investigated to date. In this study, growth rate dispersion and the change in morphology were investigated in situ and via bottle roller experiments. The surfaces of the (0 1 0) faces of crystals were examined with Atomic Force Microscopy. Smaller, slow growing crystals tend to have smaller (0 1 0) faces with narrow bases and displayed a single double spiral in the centre of the crystal with 2 nm high steps. Additional double spirals in other crystals resulted in faster growth rates. Large, fast growing crystals were observed to have larger (0 1 0) faces with fast growth in both the a and b directions (giving a broader crystal base) with macro steps parallel to the (c direction). The number and location of spirals or existence of macro steps appears to influence the crystal morphology, growth rates and growth rate dispersion in lactose crystals.
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spelling curtin-20.500.11937-170812017-09-13T15:44:14Z Investigation of growth rate dispersion in lactose crystallisation by AFM Dincer, Tuna Ogden, Mark Parkinson, Gordon B1. Organic compounds A1. Atomic force microscopy A2. Single crystal growth A1. Optical microscopy A2. Growth from solution α-Lactose monohydrate crystals have been reported to exhibit growth rate dispersion (GRD). Variation in surface dislocations has been suggested as the cause of GRD, but this has not been further investigated to date. In this study, growth rate dispersion and the change in morphology were investigated in situ and via bottle roller experiments. The surfaces of the (0 1 0) faces of crystals were examined with Atomic Force Microscopy. Smaller, slow growing crystals tend to have smaller (0 1 0) faces with narrow bases and displayed a single double spiral in the centre of the crystal with 2 nm high steps. Additional double spirals in other crystals resulted in faster growth rates. Large, fast growing crystals were observed to have larger (0 1 0) faces with fast growth in both the a and b directions (giving a broader crystal base) with macro steps parallel to the (c direction). The number and location of spirals or existence of macro steps appears to influence the crystal morphology, growth rates and growth rate dispersion in lactose crystals. 2014 Journal Article http://hdl.handle.net/20.500.11937/17081 10.1016/j.jcrysgro.2014.06.027 Elsevier fulltext
spellingShingle B1. Organic compounds
A1. Atomic force microscopy
A2. Single crystal growth
A1. Optical microscopy
A2. Growth from solution
Dincer, Tuna
Ogden, Mark
Parkinson, Gordon
Investigation of growth rate dispersion in lactose crystallisation by AFM
title Investigation of growth rate dispersion in lactose crystallisation by AFM
title_full Investigation of growth rate dispersion in lactose crystallisation by AFM
title_fullStr Investigation of growth rate dispersion in lactose crystallisation by AFM
title_full_unstemmed Investigation of growth rate dispersion in lactose crystallisation by AFM
title_short Investigation of growth rate dispersion in lactose crystallisation by AFM
title_sort investigation of growth rate dispersion in lactose crystallisation by afm
topic B1. Organic compounds
A1. Atomic force microscopy
A2. Single crystal growth
A1. Optical microscopy
A2. Growth from solution
url http://hdl.handle.net/20.500.11937/17081