Facile synthesis and electrochemical properties of octahedral gold nanocrystals

High-yield octahedral gold nanocrystals of *45 nm in size have been facilely synthesized by one-pot reduction of HAuCl4 using formic acid in cetyltrimethylammonium bromide (CTAB) aqueous solution. The results showed that CTAB can promote the formation of single-crystalline nucleation and preferentia...

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Main Authors: Wang, D., Huang, J., Liu, Yang, Han, X., You, T.
Format: Journal Article
Published: Springer Netherlands 2011
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/13655
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author Wang, D.
Huang, J.
Liu, Yang
Han, X.
You, T.
author_facet Wang, D.
Huang, J.
Liu, Yang
Han, X.
You, T.
author_sort Wang, D.
building Curtin Institutional Repository
collection Online Access
description High-yield octahedral gold nanocrystals of *45 nm in size have been facilely synthesized by one-pot reduction of HAuCl4 using formic acid in cetyltrimethylammonium bromide (CTAB) aqueous solution. The results showed that CTAB can promote the formation of single-crystalline nucleation and preferentially adsorb on the (111) planes of gold nanocrystals, resulting in the formation of octahedral gold nanocrystals. Formic acid acted as not only a mild reducing agent, but also could promote the formation of (111) facet. The octahedral gold nanocrystals exhibited similar cyclic voltammetry (CV) curves to single-crystal Au (111) electrode and excellent electrocatalytic activity for methanol oxidation. This synthetic strategy may open new route for facile synthesis of shape-controlled metal nanoparticles.
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institution Curtin University Malaysia
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last_indexed 2025-11-14T07:04:30Z
publishDate 2011
publisher Springer Netherlands
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spelling curtin-20.500.11937-136552017-09-13T15:01:41Z Facile synthesis and electrochemical properties of octahedral gold nanocrystals Wang, D. Huang, J. Liu, Yang Han, X. You, T. Nanocrystal Single-crystal Electrocatalytic activity Cyclic voltammetry Shape-control High-yield octahedral gold nanocrystals of *45 nm in size have been facilely synthesized by one-pot reduction of HAuCl4 using formic acid in cetyltrimethylammonium bromide (CTAB) aqueous solution. The results showed that CTAB can promote the formation of single-crystalline nucleation and preferentially adsorb on the (111) planes of gold nanocrystals, resulting in the formation of octahedral gold nanocrystals. Formic acid acted as not only a mild reducing agent, but also could promote the formation of (111) facet. The octahedral gold nanocrystals exhibited similar cyclic voltammetry (CV) curves to single-crystal Au (111) electrode and excellent electrocatalytic activity for methanol oxidation. This synthetic strategy may open new route for facile synthesis of shape-controlled metal nanoparticles. 2011 Journal Article http://hdl.handle.net/20.500.11937/13655 10.1007/s11051-010-0014-3 Springer Netherlands restricted
spellingShingle Nanocrystal
Single-crystal
Electrocatalytic activity
Cyclic voltammetry
Shape-control
Wang, D.
Huang, J.
Liu, Yang
Han, X.
You, T.
Facile synthesis and electrochemical properties of octahedral gold nanocrystals
title Facile synthesis and electrochemical properties of octahedral gold nanocrystals
title_full Facile synthesis and electrochemical properties of octahedral gold nanocrystals
title_fullStr Facile synthesis and electrochemical properties of octahedral gold nanocrystals
title_full_unstemmed Facile synthesis and electrochemical properties of octahedral gold nanocrystals
title_short Facile synthesis and electrochemical properties of octahedral gold nanocrystals
title_sort facile synthesis and electrochemical properties of octahedral gold nanocrystals
topic Nanocrystal
Single-crystal
Electrocatalytic activity
Cyclic voltammetry
Shape-control
url http://hdl.handle.net/20.500.11937/13655