Couples of colloidal semiconductor nanorods formed by self-limited assembly

Colloidal nanocrystal synthesis provides a powerful approach for creating unique nanostructures of relevance for applications. Here, we report that wurtzite ZnSe nanorod couples connected by twinning structures can be synthesized by means of a self-limited assembly process. Unlike for individual nan...

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Main Authors: Jia, Guohua, Sitt, A., Hitin, G., Hadar, I., Bekenstein, Y., Amit, Y., Popov, I., Banin, U.
Format: Journal Article
Published: 2014
Online Access:http://hdl.handle.net/20.500.11937/13634
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author Jia, Guohua
Sitt, A.
Hitin, G.
Hadar, I.
Bekenstein, Y.
Amit, Y.
Popov, I.
Banin, U.
author_facet Jia, Guohua
Sitt, A.
Hitin, G.
Hadar, I.
Bekenstein, Y.
Amit, Y.
Popov, I.
Banin, U.
author_sort Jia, Guohua
building Curtin Institutional Repository
collection Online Access
description Colloidal nanocrystal synthesis provides a powerful approach for creating unique nanostructures of relevance for applications. Here, we report that wurtzite ZnSe nanorod couples connected by twinning structures can be synthesized by means of a self-limited assembly process. Unlike for individual nanorods, the band-edge states calculated for the nanorod couples are predominantly confined to the short edges of the structure and this leads to low photoluminescence polarization anisotropy, as confirmed by single-particle fluorescence. Through a cation-exchange approach, the composition of nanorod couples can be readily expanded to additional materials, such as CdSe and PbSe. We anticipate that this family of nanorod-couple structures with distinct compositions and controlled properties will constitute an ideal system for the investigation of electronic coupling effects between individual nanorod components on the nanoscale, with relevance to applications in optics, photocatalysis and optoelectronic devices.
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spelling curtin-20.500.11937-136342017-09-13T15:01:02Z Couples of colloidal semiconductor nanorods formed by self-limited assembly Jia, Guohua Sitt, A. Hitin, G. Hadar, I. Bekenstein, Y. Amit, Y. Popov, I. Banin, U. Colloidal nanocrystal synthesis provides a powerful approach for creating unique nanostructures of relevance for applications. Here, we report that wurtzite ZnSe nanorod couples connected by twinning structures can be synthesized by means of a self-limited assembly process. Unlike for individual nanorods, the band-edge states calculated for the nanorod couples are predominantly confined to the short edges of the structure and this leads to low photoluminescence polarization anisotropy, as confirmed by single-particle fluorescence. Through a cation-exchange approach, the composition of nanorod couples can be readily expanded to additional materials, such as CdSe and PbSe. We anticipate that this family of nanorod-couple structures with distinct compositions and controlled properties will constitute an ideal system for the investigation of electronic coupling effects between individual nanorod components on the nanoscale, with relevance to applications in optics, photocatalysis and optoelectronic devices. 2014 Journal Article http://hdl.handle.net/20.500.11937/13634 10.1038/nmat3867 restricted
spellingShingle Jia, Guohua
Sitt, A.
Hitin, G.
Hadar, I.
Bekenstein, Y.
Amit, Y.
Popov, I.
Banin, U.
Couples of colloidal semiconductor nanorods formed by self-limited assembly
title Couples of colloidal semiconductor nanorods formed by self-limited assembly
title_full Couples of colloidal semiconductor nanorods formed by self-limited assembly
title_fullStr Couples of colloidal semiconductor nanorods formed by self-limited assembly
title_full_unstemmed Couples of colloidal semiconductor nanorods formed by self-limited assembly
title_short Couples of colloidal semiconductor nanorods formed by self-limited assembly
title_sort couples of colloidal semiconductor nanorods formed by self-limited assembly
url http://hdl.handle.net/20.500.11937/13634