Molecular Dynamics Investigation on Adsorption Layer of Alcohols at the Air/Brine Interface

Alcohols are a significant group of surfactants which have been employed extensively in industry to improve the interfacial effects. Recently, the change in surface potential (ΔV)of two isomeric hexanols, methyl isobutyl carbinol (MIBC) and 1-hexanol, was investigated by using an ionizing241Am elect...

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Main Authors: Nguyen, Van Cuong, Phan, Chi, Ang, Ming, Nakahara, H., Shibata, O., Moroi, Y.
Format: Journal Article
Published: American Chemical Society 2015
Online Access:http://hdl.handle.net/20.500.11937/10294
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author Nguyen, Van Cuong
Phan, Chi
Ang, Ming
Nakahara, H.
Shibata, O.
Moroi, Y.
author_facet Nguyen, Van Cuong
Phan, Chi
Ang, Ming
Nakahara, H.
Shibata, O.
Moroi, Y.
author_sort Nguyen, Van Cuong
building Curtin Institutional Repository
collection Online Access
description Alcohols are a significant group of surfactants which have been employed extensively in industry to improve the interfacial effects. Recently, the change in surface potential (ΔV)of two isomeric hexanols, methyl isobutyl carbinol (MIBC) and 1-hexanol, was investigated by using an ionizing241Am electrode. It clearly showed the opposite effects between MIBC and 1-hexanol in the interfacial zone: one enhanced the presence of cations, whereas the other enhanced the presence of anions. This study employs molecular dynamics simulation to provide new insights into the interactions between alcohol molecules and ions as well as water at the molecular level. The results qualitatively agreed with the experimental data and verified the significance of MIBC branching structure on the molecular arrangement within the interfacial zone. The results also highlighted the role of the second water layer on the interfacial properties.
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publishDate 2015
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spelling curtin-20.500.11937-102942017-10-02T02:28:09Z Molecular Dynamics Investigation on Adsorption Layer of Alcohols at the Air/Brine Interface Nguyen, Van Cuong Phan, Chi Ang, Ming Nakahara, H. Shibata, O. Moroi, Y. Alcohols are a significant group of surfactants which have been employed extensively in industry to improve the interfacial effects. Recently, the change in surface potential (ΔV)of two isomeric hexanols, methyl isobutyl carbinol (MIBC) and 1-hexanol, was investigated by using an ionizing241Am electrode. It clearly showed the opposite effects between MIBC and 1-hexanol in the interfacial zone: one enhanced the presence of cations, whereas the other enhanced the presence of anions. This study employs molecular dynamics simulation to provide new insights into the interactions between alcohol molecules and ions as well as water at the molecular level. The results qualitatively agreed with the experimental data and verified the significance of MIBC branching structure on the molecular arrangement within the interfacial zone. The results also highlighted the role of the second water layer on the interfacial properties. 2015 Journal Article http://hdl.handle.net/20.500.11937/10294 10.1021/la504471q American Chemical Society restricted
spellingShingle Nguyen, Van Cuong
Phan, Chi
Ang, Ming
Nakahara, H.
Shibata, O.
Moroi, Y.
Molecular Dynamics Investigation on Adsorption Layer of Alcohols at the Air/Brine Interface
title Molecular Dynamics Investigation on Adsorption Layer of Alcohols at the Air/Brine Interface
title_full Molecular Dynamics Investigation on Adsorption Layer of Alcohols at the Air/Brine Interface
title_fullStr Molecular Dynamics Investigation on Adsorption Layer of Alcohols at the Air/Brine Interface
title_full_unstemmed Molecular Dynamics Investigation on Adsorption Layer of Alcohols at the Air/Brine Interface
title_short Molecular Dynamics Investigation on Adsorption Layer of Alcohols at the Air/Brine Interface
title_sort molecular dynamics investigation on adsorption layer of alcohols at the air/brine interface
url http://hdl.handle.net/20.500.11937/10294